Major and trace element data of lava and tephra samples from the 2021 Tajogaite eruption. Major and select trace element collected by XRF, trace elements collected by ICPMS, both at the University of Granada. Data collected as part of NERC Urgency Grant led by K Chamberlain (Liverpool), in collaboration with M Pankhurst (INVOLCAN), J Scarrow (Granada), D Morgan (Leeds), J Hickey (Exeter), D Neave (Manchester), for understanding how eruptions begin, evolve and end. Samples analysed span the entire September - December 2021 eruptive sequence of Tajogaite, and data were collected between December 2021 and August 2022.